Lithium Metal Anode Materials Design: Interphase and Host

doi:10.1007/s41918-019-00054-2

Electrochemical Energy Reviews ›› 2019, Vol. 2 ›› Issue (4): 509-517.doi: 10.1007/s41918-019-00054-2

• PERSPECTIVE • 下一篇

Lithium Metal Anode Materials Design: Interphase and Host

Hansen Wang¹, Yayuan Liu¹, Yuzhang Li¹, Yi Cui^1,2

1 Department of Materials Science and Engineering, Stanford University, Stanford, CA 94305, USA;
2 Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA

收稿日期:2019-02-10 修回日期:2019-04-23 出版日期:2019-12-20 发布日期:2020-03-28
通讯作者: Yi Cui E-mail:yicui@stanford.edu
基金资助:
We acknowledge the support from the Assistant Secretary for Energy Efciency and Renewable Energy, Ofce of Vehicle Technologies, Battery Materials Research (BMR) and Battery 500 Program of the US Department of Energy. Yayuan L. acknowledges the support from Stanford University through the Stanford Graduate Fellowship. Yuzhang L. acknowledges the Intelligence Community Fellowship for funding.

Lithium Metal Anode Materials Design: Interphase and Host

Hansen Wang¹, Yayuan Liu¹, Yuzhang Li¹, Yi Cui^1,2

1 Department of Materials Science and Engineering, Stanford University, Stanford, CA 94305, USA;
2 Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA

Received:2019-02-10 Revised:2019-04-23 Online:2019-12-20 Published:2020-03-28
Contact: Yi Cui E-mail:yicui@stanford.edu
Supported by:
We acknowledge the support from the Assistant Secretary for Energy Efciency and Renewable Energy, Ofce of Vehicle Technologies, Battery Materials Research (BMR) and Battery 500 Program of the US Department of Energy. Yayuan L. acknowledges the support from Stanford University through the Stanford Graduate Fellowship. Yuzhang L. acknowledges the Intelligence Community Fellowship for funding.

摘要/Abstract

摘要：

Li metal is the ultimate anode choice due to its highest theoretical capacity and lowest electrode potential, but it is far from practical applications with its poor cycle lifetime. Recent research progresses show that materials designs of interphase and host structures for Li metal are two efective ways addressing the key issues of Li metal anodes. Despite the exciting improvement on Li metal cycling capability, problems still exist with these methodologies, such as the defcient long-time cycling stability of interphase materials and the accelerated Li corrosion for high surface area three-dimensional composite Li anodes. As a result, Coulombic efciency of Li metal is still not sufcient for full-cell cycling. In the near future, an interphase protected three-dimensional composite Li metal anode, combined with high performance novel electrolytes might be the ultimate solution. Besides, nanoscale characterization technologies are also vital for guiding future Li metal anode designs.

Full-text：https://link.springer.com/article/10.1007/s41918-019-00054-2

关键词: Lithium metal anode, Interphase, Host, Electrolyte, Cryo-EM

Abstract:

Full-text：https://link.springer.com/article/10.1007/s41918-019-00054-2

Key words: Lithium metal anode, Interphase, Host, Electrolyte, Cryo-EM

Hansen Wang, Yayuan Liu, Yuzhang Li, Yi Cui. Lithium Metal Anode Materials Design: Interphase and Host[J]. Electrochemical Energy Reviews, 2019, 2(4): 509-517.

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Lithium Metal Anode Materials Design: Interphase and Host

Lithium Metal Anode Materials Design: Interphase and Host

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