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Electrochemical Energy Reviews ›› 2024, Vol. 7 ›› Issue (4): 34-.doi: 10.1007/s41918-024-00234-9

• • 上一篇    下一篇

The Origin, Characterization, and Precise Design and Regulation of Diverse Hard Carbon

Junjie Liu1, Ling Huang1, Huiqun Wang1, Liyuan Sha1, Miao Liu1, Zhefei Sun1, Jiawei Gu1, Haodong Liu3, Jinbao Zhao1, Qiaobao Zhang1,2,4, Li Zhang1   

  1. 1. State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, College of Materials, Tan Kah Kee Innovation Laboratory, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM), Xiamen University, Xiamen 361005, Fujian, China;
    2. Longmen Laboratory, Luoyang 471023, Henan, China;
    3. Center for Memory and Recording Research Building, UC San Diego, La Jolla, CA 92093, USA;
    4. Shenzhen Research Institute of Xiamen University, Shenzhen 518000, Guangdong, China
  • 收稿日期:2024-05-27 修回日期:2024-07-24 出版日期:2024-12-20 发布日期:2024-12-28
  • 通讯作者: Qiaobao Zhang,E-mail:zhangqiaobao@xmu.edu.cn;Li Zhang,E-mail:zhangli81@xmu.edu.cn E-mail:zhangqiaobao@xmu.edu.cn;zhangli81@xmu.edu.cn
  • 基金资助:
    This work was supported by the National Natural Science Foundation of China (Grant Nos.92372101,52122211,52072323 and 21875155),the Fundamental Research Funds for the Central Universities (No.20720220010),the National Key Research and Development Program of China (No.2021YFA1201502),the Frontier Exploration Projects of Longmen Laboratory (grant No.LMQYTSKT008) and the Shenzhen Technical Plan Project (No.JCYJ20220818101003008).L.Zhang and Q.B.Zhang acknowledge the support of Nanqiang Young Top-notch Talent Fellowship in Xiamen University.We also thank Prof.Zhaowu Tian in Department of Chemistry,Xiamen University for his helpful guidance.

The Origin, Characterization, and Precise Design and Regulation of Diverse Hard Carbon

Junjie Liu1, Ling Huang1, Huiqun Wang1, Liyuan Sha1, Miao Liu1, Zhefei Sun1, Jiawei Gu1, Haodong Liu3, Jinbao Zhao1, Qiaobao Zhang1,2,4, Li Zhang1   

  1. 1. State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, College of Materials, Tan Kah Kee Innovation Laboratory, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM), Xiamen University, Xiamen 361005, Fujian, China;
    2. Longmen Laboratory, Luoyang 471023, Henan, China;
    3. Center for Memory and Recording Research Building, UC San Diego, La Jolla, CA 92093, USA;
    4. Shenzhen Research Institute of Xiamen University, Shenzhen 518000, Guangdong, China
  • Received:2024-05-27 Revised:2024-07-24 Online:2024-12-20 Published:2024-12-28
  • Contact: Qiaobao Zhang,E-mail:zhangqiaobao@xmu.edu.cn;Li Zhang,E-mail:zhangli81@xmu.edu.cn E-mail:zhangqiaobao@xmu.edu.cn;zhangli81@xmu.edu.cn
  • Supported by:
    This work was supported by the National Natural Science Foundation of China (Grant Nos.92372101,52122211,52072323 and 21875155),the Fundamental Research Funds for the Central Universities (No.20720220010),the National Key Research and Development Program of China (No.2021YFA1201502),the Frontier Exploration Projects of Longmen Laboratory (grant No.LMQYTSKT008) and the Shenzhen Technical Plan Project (No.JCYJ20220818101003008).L.Zhang and Q.B.Zhang acknowledge the support of Nanqiang Young Top-notch Talent Fellowship in Xiamen University.We also thank Prof.Zhaowu Tian in Department of Chemistry,Xiamen University for his helpful guidance.

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摘要： Hard carbon, a prominent member of carbonaceous materials, shows immense potential as a high-performance anode for energy storage in batteries, attracting significant attention. Its structural diversity offers superior performance and high tunability, making it ideal for use as an anode in lithium-ion batteries, sodium-ion batteries, and potassium-ion batteries. To develop higher-performance hard carbon anode materials, extensive research has been conducted to understand the storage mechanisms of alkali metal ions in hard carbon. Building on this foundation, this paper provides an in-depth review of the relationship between the structure of hard carbon and its electrochemical properties with alkali metal ions. It emphasizes the structural design and characterization of hard carbon, the storage mechanisms of alkali metal ions, and key strategies for structural modulation. Additionally, it offers a forward-looking perspective on the future potential of hard carbon. This review aims to provide a comprehensive overview of the current state of hard carbon anodes in battery research and highlights the promising future of this rapidly evolving field in advancing the development of next-generation alkali metal-ion batteries.

关键词: Hard carbon, Alkali metal ion batteries, Structure design strategy, Electrochemical energy storage, Storage Mechanism

Abstract: Hard carbon, a prominent member of carbonaceous materials, shows immense potential as a high-performance anode for energy storage in batteries, attracting significant attention. Its structural diversity offers superior performance and high tunability, making it ideal for use as an anode in lithium-ion batteries, sodium-ion batteries, and potassium-ion batteries. To develop higher-performance hard carbon anode materials, extensive research has been conducted to understand the storage mechanisms of alkali metal ions in hard carbon. Building on this foundation, this paper provides an in-depth review of the relationship between the structure of hard carbon and its electrochemical properties with alkali metal ions. It emphasizes the structural design and characterization of hard carbon, the storage mechanisms of alkali metal ions, and key strategies for structural modulation. Additionally, it offers a forward-looking perspective on the future potential of hard carbon. This review aims to provide a comprehensive overview of the current state of hard carbon anodes in battery research and highlights the promising future of this rapidly evolving field in advancing the development of next-generation alkali metal-ion batteries.

Key words: Hard carbon, Alkali metal ion batteries, Structure design strategy, Electrochemical energy storage, Storage Mechanism

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