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Electrochemical Energy Reviews ›› 2025, Vol. 8 ›› Issue (3): 19-.doi: 10.1007/s41918-025-00258-9

• • 上一篇    

Interlayer Nanoarchitecture Modification of Layered Materials in Rechargeable Metal-Ion Batteries

Yuchen Wang1,2, Huiyan Feng2,3, Chengzhi Zhang2, Quanbin Liu3, Jun Tan1,2,4, Chong Ye1   

  1. 1. Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology, College of Materials Science and Engineering, Hunan University, Changsha 410082, Hunan, China;
    2. Ji Hua Laboratory, Foshan 528000, Guangdong China;
    3. School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, Guangdong, China;
    4. Foshan University, Foshan 528000, Guangdong, China
  • 收稿日期:2024-11-04 修回日期:2025-01-25 出版日期:2025-09-20 发布日期:2025-11-12
  • 通讯作者: Chengzhi Zhang Email:E-mail:zhangchz@jihualab.ac.cn;Chong Ye Email:E-mail:yec@hnu.edu.cn E-mail:zhangchz@jihualab.ac.cn;yec@hnu.edu.cn
  • 基金资助:
    Yuchen Wang and Huiyan Feng contributed equally to this work. This project was supported by the National Natural Science Foundation of China (No. 22309062), the Guangdong Basic and Applied Basic Research Foundation (No. 2022A1515110052), and the Jihua Laboratory (No. X200191TL200).

Interlayer Nanoarchitecture Modification of Layered Materials in Rechargeable Metal-Ion Batteries

Yuchen Wang1,2, Huiyan Feng2,3, Chengzhi Zhang2, Quanbin Liu3, Jun Tan1,2,4, Chong Ye1   

  1. 1. Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology, College of Materials Science and Engineering, Hunan University, Changsha 410082, Hunan, China;
    2. Ji Hua Laboratory, Foshan 528000, Guangdong China;
    3. School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, Guangdong, China;
    4. Foshan University, Foshan 528000, Guangdong, China
  • Received:2024-11-04 Revised:2025-01-25 Online:2025-09-20 Published:2025-11-12
  • Contact: Chengzhi Zhang Email:E-mail:zhangchz@jihualab.ac.cn;Chong Ye Email:E-mail:yec@hnu.edu.cn E-mail:zhangchz@jihualab.ac.cn;yec@hnu.edu.cn
  • Supported by:
    Yuchen Wang and Huiyan Feng contributed equally to this work. This project was supported by the National Natural Science Foundation of China (No. 22309062), the Guangdong Basic and Applied Basic Research Foundation (No. 2022A1515110052), and the Jihua Laboratory (No. X200191TL200).

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摘要： In this new era of energy, a tendency to increase the power density and capacity of advanced rechargeable batteries is urgently needed. With research on metal-ion (Li+, Na+, K+, Zn2+, Mg2+, and Al3+) batteries based on and beyond rocking-chair mechanism development, more attention has been given to modification of electrode materials. Layered materials, along with their two-dimensional (2D) analogs, show remarkable superiority in ion-intercalation chemistry and modification feasibility. In this context, extensive experimental and theoretical studies have been conducted in the design of interlayer nanoarchitectures to optimize their electrochemical performance. This review provides a comprehensive summary of the modification strategies for the interlayer nanostructure of layered materials, reveals the relationships between the inserted species and electrochemical performance, and offers guidance on the modification parameters for various metal-ion batteries. Finally, an outlook of the application potential, future research directions, and remaining challenges is provided. Overall, this review underscores the importance of material modification in achieving high-power density and high-capacity electrodes for batteries, paving the way for significant advancements in energy storage technology.

关键词: Layered materials, Interlayer modulation, Rechargeable batteries, Energy storage technology

Abstract: In this new era of energy, a tendency to increase the power density and capacity of advanced rechargeable batteries is urgently needed. With research on metal-ion (Li+, Na+, K+, Zn2+, Mg2+, and Al3+) batteries based on and beyond rocking-chair mechanism development, more attention has been given to modification of electrode materials. Layered materials, along with their two-dimensional (2D) analogs, show remarkable superiority in ion-intercalation chemistry and modification feasibility. In this context, extensive experimental and theoretical studies have been conducted in the design of interlayer nanoarchitectures to optimize their electrochemical performance. This review provides a comprehensive summary of the modification strategies for the interlayer nanostructure of layered materials, reveals the relationships between the inserted species and electrochemical performance, and offers guidance on the modification parameters for various metal-ion batteries. Finally, an outlook of the application potential, future research directions, and remaining challenges is provided. Overall, this review underscores the importance of material modification in achieving high-power density and high-capacity electrodes for batteries, paving the way for significant advancements in energy storage technology.

Key words: Layered materials, Interlayer modulation, Rechargeable batteries, Energy storage technology

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