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Electrochemical Energy Reviews ›› 2024, Vol. 7 ›› Issue (3): 26-.doi: 10.1007/s41918-024-00223-y

所属专题： Electrochemical Nanomaterials

• • 上一篇    下一篇

Nanoporous Carbon Materials Derived from Biomass Precursors: Sustainable Materials for Energy Conversion and Storage

Zhikai Chen1,2, Xiaoli Jiang1,2, Yash Boyjoo3,7, Lan Zhang8, Wei Li1, Lin Zhao1, Yanxia Liu1,2, Yagang Zhang1,2, Jian Liu3,5,6, Xifei Li4   

  1. 1. School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 611731, Sichuan, China;
    2. State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 611731, Sichuan, China;
    3. State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
    4. School of Materials Science and Engineering, Xi'an University of Technology, Xi'an 710048, Shaanxi, China;
    5. DICP-Surrey Joint Centre for Future Materials, Department of Chemical and Process Engineering and Advanced Technology Institute, University of Surrey, Guilford, Surrey GU27XH, UK;
    6. College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, Inner Mongolia, China;
    7. Curtin Mauritius, Telfair, 80809, Moka, Mauritius;
    8. Univ Lyon, CNRS, INSA-Lyon, Université Claude Bernard Lyon 1, CETHIL UMR5008, 69621 Villeurbanne, France
  • 收稿日期:2023-05-28 修回日期:2024-02-01 出版日期:2024-09-20 发布日期:2024-09-23
  • 通讯作者: Yagang Zhang,E-mail:ygzhang@uestc.edu.cn;Jian Liu,E-mail:jianliu@surrey.ac.uk;Xifei Li,E-mail:xfli@xaut.edu.cn E-mail:jianliu@surrey.ac.uk;ygzhang@uestc.edu.cn;jianliu@surrey.ac.uk;xfli@xaut.edu.cn
  • 基金资助:
    This research was financially supported by Key Research and Development Projects of Sichuan Province (2023YFG0222), “Tianfu Emei” Science and Technology Innovation Leader Program in Sichuan Province, University of Electronic Science and Technology of China Talent Start-up Funds (A1098 5310 2360 1208), and National Natural Science Foundation of China (21472235, 21464015).

Nanoporous Carbon Materials Derived from Biomass Precursors: Sustainable Materials for Energy Conversion and Storage

Zhikai Chen1,2, Xiaoli Jiang1,2, Yash Boyjoo3,7, Lan Zhang8, Wei Li1, Lin Zhao1, Yanxia Liu1,2, Yagang Zhang1,2, Jian Liu3,5,6, Xifei Li4   

  1. 1. School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 611731, Sichuan, China;
    2. State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 611731, Sichuan, China;
    3. State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;
    4. School of Materials Science and Engineering, Xi'an University of Technology, Xi'an 710048, Shaanxi, China;
    5. DICP-Surrey Joint Centre for Future Materials, Department of Chemical and Process Engineering and Advanced Technology Institute, University of Surrey, Guilford, Surrey GU27XH, UK;
    6. College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, Inner Mongolia, China;
    7. Curtin Mauritius, Telfair, 80809, Moka, Mauritius;
    8. Univ Lyon, CNRS, INSA-Lyon, Université Claude Bernard Lyon 1, CETHIL UMR5008, 69621 Villeurbanne, France
  • Received:2023-05-28 Revised:2024-02-01 Online:2024-09-20 Published:2024-09-23
  • Contact: Yagang Zhang,E-mail:ygzhang@uestc.edu.cn;Jian Liu,E-mail:jianliu@surrey.ac.uk;Xifei Li,E-mail:xfli@xaut.edu.cn E-mail:jianliu@surrey.ac.uk;ygzhang@uestc.edu.cn;jianliu@surrey.ac.uk;xfli@xaut.edu.cn
  • Supported by:
    This research was financially supported by Key Research and Development Projects of Sichuan Province (2023YFG0222), “Tianfu Emei” Science and Technology Innovation Leader Program in Sichuan Province, University of Electronic Science and Technology of China Talent Start-up Funds (A1098 5310 2360 1208), and National Natural Science Foundation of China (21472235, 21464015).

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摘要： Biomass, which is derived from abundant renewable resources, is a promising alternative to fossil-fuel-based carbon materials for building a green and sustainable society. Biomass-based carbon materials (BCMs) with tailored hierarchical pore structures, large specific surface areas, and various surface functional groups have been extensively studied as energy and catalysis-related materials. This review provides insights from the perspectives of intrinsic physicochemical properties and structure-property relationships for discussing several fundamental yet significant issues in BCMs and their consequences. First, the synthesis, properties, and influencing factors of BCMs are discussed. Then, the causes and effects of the poor mechanical properties of biochar are explored. The factors affecting the properties of BCMs are presented, and the approaches for tuning these properties of biochar are summarized. Further, the applications of BCMs in energy storage and conversion are highlighted, including hydrogen storage and production, fuel cells, supercapacitors, hybrid electrodes, catalytic reforming, oxygen and CO2 reduction, and acetylene hydrochlorination. Finally, the future trends and prospects for biochar are proposed. This review aims to serve as a useful, up-to-date reference for future studies on BCMs for energy and catalytic applications.

关键词: Nanoporous carbon materials, Biomass-based sustainable materials, Energy storage, Energy conversion

Abstract: Biomass, which is derived from abundant renewable resources, is a promising alternative to fossil-fuel-based carbon materials for building a green and sustainable society. Biomass-based carbon materials (BCMs) with tailored hierarchical pore structures, large specific surface areas, and various surface functional groups have been extensively studied as energy and catalysis-related materials. This review provides insights from the perspectives of intrinsic physicochemical properties and structure-property relationships for discussing several fundamental yet significant issues in BCMs and their consequences. First, the synthesis, properties, and influencing factors of BCMs are discussed. Then, the causes and effects of the poor mechanical properties of biochar are explored. The factors affecting the properties of BCMs are presented, and the approaches for tuning these properties of biochar are summarized. Further, the applications of BCMs in energy storage and conversion are highlighted, including hydrogen storage and production, fuel cells, supercapacitors, hybrid electrodes, catalytic reforming, oxygen and CO2 reduction, and acetylene hydrochlorination. Finally, the future trends and prospects for biochar are proposed. This review aims to serve as a useful, up-to-date reference for future studies on BCMs for energy and catalytic applications.

Key words: Nanoporous carbon materials, Biomass-based sustainable materials, Energy storage, Energy conversion

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